Reconfigurable Transport and Assembly of Colloidal Particles via Opto-Chemical-Electronic Tweezer (OCET) (2025)

    Surfaces, Interfaces, and Applications

    • Xi Chen*

      Xi Chen

      College of Materials and Chemistry & Chemical Engineering, Chengdu University of Technology, Chengdu, Sichuan 610059, China

      School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen, Guangdong 518055, China

      *Email: [emailprotected]

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    • Shifang Duan

      Shifang Duan

      School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen, Guangdong 518055, China

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    • Dezhou Cao

      Dezhou Cao

      School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen, Guangdong 518055, China

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    • Jinyao Tang

      Jinyao Tang

      Department of Chemistry, The University of Hong Kong, Hong Kong 999077, China

      HKU-CAS Joint Laboratory on New Materials and Department of Chemistry, Hong Kong 999077, China

      State Key Laboratory of Synthetic Chemistry, The University of Hong Kong, Hong Kong 999077, China

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    • Xing Ma

      Xing Ma

      School of Integrated Circuits, Harbin Institute of Technology (Shenzhen), Shenzhen 518055, China

      Sauvage Laboratory for Smart Materials, School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen 518055, China

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    • Ting Kuang

      Ting Kuang

      Education Center of Experiments and Innovations, Harbin Institute of Technology (Shenzhen), Shenzhen 518055, China

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    • Shuailong Zhang

      Shuailong Zhang

      School of Integrated Circuits and Electronics, Beijing Institute of Technology, Beijing 100081, China

      Chongqing Institute of Microelectronics and Microsystems, Beijing Institute of Technology, Chongqing 400000, China

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    • Wei Wang*

      Wei Wang

      School of Materials Science and Engineering, Harbin Institute of Technology (Shenzhen), Shenzhen, Guangdong 518055, China

      *Email: [emailprotected]

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    Other Access OptionsSupporting Information (6)

    ACS Applied Materials & Interfaces

    Cite this: ACS Appl. Mater. Interfaces 2025, XXXX, XXX, XXX-XXX

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    https://pubs.acs.org/doi/10.1021/acsami.5c02233

    Published April 22, 2025

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    Reconfigurable Transport and Assembly of Colloidal Particles via Opto-Chemical-Electronic Tweezer (OCET) (7)

    Transporting and assembling colloidal particles is key to applications such as drug delivery, the fabrication of functional materials, and microrobotics. As a result, there is intense effort in developing techniques for manipulating colloids at high spatial and temporal resolutions, and in a dynamic, reconfigurable manner. Although optical manipulation provides precise particle control, its application is often limited by high energy requirements and intricate setups. In this study, we present an opto-chemical-electronic tweezer (OCET), a novel particle manipulation strategy that addresses these limitations. The OCET system utilizes a photocatalytic TiO2/Pt film irradiated with perpendicular UV light. An electric field is then generated parallel to the film at the boundary of the patterned UV light, directed from the illuminated region to the dark region. The consequent electrophoresis and electroosmosis work in tandem to move inert colloidal particles (e.g., SiO2 microspheres) at ∼1 μm/s and trap them a few μm inside the illuminated region along the boundary of the light pattern. By dynamically modulating light patterns, the OCET system achieves directional particle transport and reconfigurable colloidal assembly into arbitrary patterns. The OCET system holds promise for applications in optofluidics, micro/nanorobotics, and biomedical systems, setting the stage for further advancements in optical manipulation technologies.

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    • Colloidal particles
    • Electric fields
    • Light
    • Oxides
    • Platinum

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    ACS Applied Materials & Interfaces

    Cite this: ACS Appl. Mater. Interfaces 2025, XXXX, XXX, XXX-XXX

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    Published April 22, 2025

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